Bentonite is a layered material that can be modified through pillarization to improve its physicochemical properties. This study aims to synthesize and characterize Ni–Mo bimetallic catalysts on aluminum pillared bentonite (BPILC) and to study the effect of variations in Ni–Mo composition. Synthesis was carried out through pillarization with Al₁₃ polycation, followed by impregnation of …